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Chinese Journal of Chemistry | Vol., Issue. | 2020-04-17 | Pages

Oxidative Dehydrogenative Silylation‐Alkenation Reaction of Alkyl Aromatics with Silanes

Wei Jiang Congde Huo Yongxin Zhang Ying Fu Xiazhen Bao Yingpeng Su

Abstract

A Cu(OAc)2/DDQ/DTBP/Py system catalyzed oxidative dehydrogenative silylation‐alkenation tandem reaction of readily available alkyl aromatic compounds with silanes was established. A variety of functionalized alkenyl organosilicon compounds were provided in good to high yields with a total β‐(E) selectivity. The control experiments revealed that the transformation might proceed through a radical pathway.

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Oxidative Dehydrogenative Silylation‐Alkenation Reaction of Alkyl Aromatics with Silanes

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Keywords

dehydrogenative

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Wei Jiang, Congde Huo, Yongxin Zhang, Ying Fu, Xiazhen Bao, Yingpeng Su,.Oxidative Dehydrogenative Silylation‐Alkenation Reaction of Alkyl Aromatics with Silanes. (),.

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